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Definition of unbound : 1. imp. & p. p. of Unbind.
2. of Unbind

Synonyms:

looseleaf, loose, untethered, unshackled

eased, freed

disconnected, broke, diverged, disjoined, dispersed, loosened, broken, detached, unfastened

unstapled, ungirt, unwrapped, unstitched

unchained, unfettered, disencumbered, disentwined, released, disentangled, reprieved, liberated, emancipated, unrestricted, free, untied, wide-open, unleashed

Usage examples:

• His companions followed the colonel's example, and begged to be allowed to die with eyes unbound. - "The Three Lieutenants", W.H.G. Kingston.
• And yet four or five fluffy little jays, that look as if they were dressed in gray fur, emerge from the eggs before the spring sunshine has unbound the icy rivers or melted the snowdrifts piled high around the evergreens. - "Bird-Neighbors", Blanchan, Neltje.
• He remained silent as the Shawnees unbound his feet. - "Spotted Deer", Elmer Gregor.