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Definition of exasperation : 1. Increase of violence or malignity; aggravation; exacerbation.
2. The act of exasperating or the state of being exasperated; irritation; keen or bitter anger.

Synonyms:

offense, fury, bothering, wrath, temper, animosity, peevishness, anger, impatience, passion, pain, rage, pettishness, choler, pestering, botheration, feelings, fretfulness

exacerbation, provocation, perturbation, indignation, aggravation, petulance, ire, harassment, discomposure, bother, trouble, scorn, pique, virulence, arousal, disturbance, inflammation, enragement, resentment, vexation, torment, bedevilment, annoyance, irritation

disgruntlement, misery, gloominess, disquiet, angst, inquietude, ennui, displeasure, despondence, cheerlessness, uneasiness, sourness, joylessness, wretchedness, anxiety, discomfort, dissatisfaction, discontent, non-satisfaction, unhappiness, uncomfortableness, boredom, anguish, frustration

Usage examples:

• Gray was checked less by the exasperation, by the authority in the speaker's tone, than by the fact that the entire complexion of the affair had changed. - "Flowing Gold", Rex Beach.
• Her grandfather turned to her, almost beside himself with exasperation. - "North, South and Over the Sea", M.E. Francis (Mrs. Francis Blundell).
• Leda asked in sudden exasperation. - "Unwise Child", Gordon Randall Garrett.